论文标题
对单层过渡金属二分法元素中磁符号的热效应
Thermal effect on magnetoexciton energy spectra in monolayer transition metal dichalcogenides
论文作者
论文摘要
广泛理解的是,温度可能会导致声子脱落,从而增强了能级的线宽并导致一些频谱变化。但是,在本文中,我们提出了一种不同的机制,该机制允许激子的质量中心(C.M.)的热运动影响单层二甲化合物(TMDCS)中的磁性exciton能量。通过C.M.的非平凡但精确的分离来自具有磁场的单层TMDC中激子的运动,我们获得了一个相对运动的方程,该方程包含与C.M.假膜体与激子气体的温度有关,但在先前的研究中被忽略。求解schrödinger方程而不省略室温下的运动型电势,显示出激子能量中的大约几个MEV热磁性移位,足以实现实验性检测。此外,这种热效应会导致激子半径和磁管系数的变化,并因此增强了激子寿命。出人意料的是,热诱导的运动型电势破坏了系统的SO(2)对称性,除了$ S $状态的室温下,在室温下在室温下进行了新的峰。该机制可以扩展到其他磁夸西颗粒(例如Trions和Biexcitons)。
It is widely comprehended that temperature may cause phonon-exciton scattering, enhancing the energy level's linewidth and leading to some spectrum shifts. However, in the present paper, we suggest a different mechanism that allows the thermal motion of the exciton's center of mass (c.m.) to affect the magnetoexciton energies in monolayer dichalcogenides (TMDCs). By the nontrivial but precise separation of the c.m. motion from an exciton in a monolayer TMDC with a magnetic field, we obtain an equation for the relative motion containing a motional Stark term proportional to the c.m. pseudomomentum, related to the temperature of the exciton gas but neglected in the previous studies. Solving the Schrödinger equation without omitting the motional Stark potential at room temperature shows approximately a few meV thermal-magnetic shifts in the exciton energies, significant enough for experimental detection. Moreover, this thermal effect causes a change in exciton radius and diamagnetic coefficient and enhances the exciton lifetime as a consequence. Surprisingly, the thermoinduced motional Stark potential breaks the system's SO(2) symmetry, conducting new peaks in the exciton absorption spectra at room temperature besides those of the $s$ states. This mechanism could be extended for other magnetoquasiparticles such as trions and biexcitons.