论文标题
长距离连续甲烷排放用双频率梳光谱监测:复杂排放场景中的部署和盲测
Long Distance Continuous Methane Emissions Monitoring with Dual Frequency Comb Spectroscopy: deployment and blind testing in complex emissions scenarios
论文作者
论文摘要
不断对石油和天然气基础设施的监测是通过快速识别和修复排放源,尤其是负责大部分总排放的大型来源来改善排放和安全性。我们先前已经证明了双频谱光谱法(DC)以及大气建模和反转技术(DCS观测系统)是一种可行而准确的方法,可在超过1 km的受控,稳定的排放情况下,以检测,归因和量化甲烷排放的距离。在这里,我们介绍了旨在模仿石油和天然气生产中运营井垫排放的复杂性的验证测试结果,以及在活性油和天然气设施中的首次现场测量。验证测试是在甲烷排放技术评估中心(METEC)测试设施上进行单盲(测量和数据分析团队的信息)。它们由一系列场景组成,范围从单个,稳定的发射点到包括间歇性发行的多个发射点(METEC“ R2”测试)。此外,我们在活动的天然气存储设施上介绍现场测量,表明该系统可以在真正的工业环境中远程自主监测甲烷排放。该字段验证是一种旨在连续和长期表征操作和逃犯的配置的配置。这些示范证实,DCS观察系统可以高信地对天然气基础设施中复杂的运营设施的排放持续监测。
Continuous monitoring of oil and gas infrastructure is of interest for improving emissions and safety by enabling rapid identification and repair of emission sources, especially large sources that are responsible for the bulk of total emissions. We have previously demonstrated dual frequency comb spectroscopy (DCS) coupled with atmospheric modeling and inversion techniques (the DCS Observing System) as a viable and accurate approach for detection, attribution and quantification of methane emissions at distances of more than 1 km under controlled, steady emissions scenarios. Here, we present the results of validation testing designed to mimic the complexity of operational well pad emissions from oil and gas production, and the first field measurements at an active oil and gas facility. The validation tests are performed single-blind (the measurement and data analysis team are not given information about the emissions) at the Methane Emissions Technology Evaluation Center (METEC) test facility. They consist of a series of scenarios ranging from a single, steady-rate emission point to multiple emission points that include intermittent releases (the METEC "R2" tests). Additionally, we present field measurements at an active natural gas storage facility demonstrating that the system can remotely and autonomously monitor methane emissions in a true industrial setting. This field verification is in a configuration designed for continuous and long-term characterization of operational and fugitive emissions. These demonstrations confirm that the DCS Observing System can provide high-confidence continuous monitoring of emissions from complex, operational facilities among natural gas infrastructure.