论文标题
重建的MOS $ _2 $Moiré超级晶格中的声子重新归一化
Phonon Renormalization in Reconstructed MoS$_2$ Moiré Superlattices
论文作者
论文摘要
在通过堆叠范德华(VDW)材料形成的Moiré晶体中,可以通过扭曲角度的细微变化来实现多样化的相关电子相和光学性能。在这里,我们发现声子光谱在MOS $ _2 $扭曲的双层中也被重新归一致,为Moiré物理学增添了新的视角。在各个小扭曲角度上,由于不同的声子模式和Moiré模式的原子重建之间的超强耦合,声子光谱迅速发展。我们为声子开发了一种新的低能连续体模型,该模型克服了计算大型Moiré超级电池的特性的杰出挑战,并成功捕获了基本的实验观察结果。值得注意的是,简单的光谱实验可以提供有关具有纳米尺寸超级细胞的Moiré晶体中应变和晶格失真的信息。新开发的理论促进了对Moiré超晶格的结构,光学和电子特性的全面和统一的理解。
In moiré crystals formed by stacking van der Waals (vdW) materials, surprisingly diverse correlated electronic phases and optical properties can be realized by a subtle change in the twist angle. Here, we discover that phonon spectra are also renormalized in MoS$_2$ twisted bilayers, adding a new perspective to moiré physics. Over a range of small twist angles, the phonon spectra evolve rapidly due to ultra-strong coupling between different phonon modes and atomic reconstructions of the moiré pattern. We develop a new low-energy continuum model for phonons that overcomes the outstanding challenge of calculating properties of large moiré supercells and successfully captures essential experimental observations. Remarkably, simple optical spectroscopy experiments can provide information on strain and lattice distortions in moiré crystals with nanometer-size supercells. The newly developed theory promotes a comprehensive and unified understanding of structural, optical, and electronic properties of moiré superlattices.