论文标题

通过RUO $ _2 $纳米线探测热活化的原子和纳米晶体缺陷运动

Probing Thermally Activated Atomic and Nanocrystalline Defect Motion through Noise Processes in RuO$_2$ Nanowires

论文作者

Yeh, Sheng-Shiuan, Yu, Cheng-Ya, Lee, Yi-Te, Chiu, Shao-Pin, Lin, Juhn-Jong

论文摘要

当今的纳米覆盖尺寸不断收缩,目的是延长摩尔定律。随着缩小尺寸的持续存在,导致低频噪声和结构不稳定性的不良动态缺陷在限制微型设备的最终性能和可靠性方面发挥了不利作用。良好的理解和对缺陷动力学的有意义的控制成为基本和紧迫的问题。在这里,我们报告了热活化的原子缺陷运动以及通过金属RUO $ _2 $ _2 $金融纳米线中的电噪声过程的纳米晶缺损运动的观察结果。首先,我们提取移动原子缺陷(氧空位)的能量分布函数和数量密度。其次,我们获得了几何大小,晶粒结合强度和动态纳米晶体的松弛时间。我们的结果清楚地表明了对纳米结构和纳米材料的有效和无创特征的强大探针,有关机械硬度,分解电流密度和/或电阻噪声的定量信息至关重要。

The present-day nanodevice dimensions continuously shrink, with the aim to prolong Moore's law. As downsizing meticulously persists, undesirable dynamic defects, which cause low-frequency noise and structural instability, play detrimental roles on limiting the ultimate performance and reliability of miniaturized devices. A good understanding and a meaningful control of the defect kinetics then become fundamental and urgent issues. Here we report observations of thermally activated atomic defect motion as well as nanocrystalline defect motion through electrical noise processes in metallic RuO$_2$ rutile nanowires around room temperature. First, we extract the energy distribution function and the number density of mobile atomic defects (oxygen vacancies). Second, we obtain the geometrical size, grain-boundary bonding strength, and relaxation times of dynamic nanocrystallites. Our results show clearly a powerful probe for effective and noninvasive characterizations of nanostructures and nanomaterials for which quantitative information about mechanical hardness, breakdown current density, and/or resistance noise is essential.

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